Document Type

Article

Publication Date

10-30-2000

Abstract

IR-visible sum-frequency generation(SFG) spectroscopy has been used in a total internal reflection geometry to study the molecular structure of polystyrene (PS) at PS/sapphire and PS/air interfaces, simultaneously. The symmetric vibrational modes of the phenyl rings dominate the SFG spectra at the PS/air interface as compared to the antisymmetric vibrational modes at the PS/sapphire interface. This indicates approximately parallel orientation of the phenyl rings at the PS/air interface while nearly perpendicular orientation at the PS/sapphire interface, with respect to the surface normal.

Publication Title

Physical Review Letters

Volume

85

Issue

18

First Page

3854

Last Page

3857

Required Publisher's Statement

Copyright 2000 American Physical Society. The original published version of this article may be found at http://dx.doi.org/10.1103/PhysRevLett.85.3854.

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