College

College of Engineering and Polymer Science

Date of Last Revision

2025-04-26 11:47:34

Major

Chemical Engineering

Honors Course

CHEE 497-001

Number of Credits

3

Degree Name

Bachelor of Science

Date of Expected Graduation

Spring 2025

Abstract

Catalytic hydrocracking was studied as a chemical recycling method for converting mixed plastic polypropylene (PP) and polyvinyl chloride (PVC) waste into sustainable aviation fuel-range hydrocarbons. Addressing both plastic pollution and aviation-related CO₂ emissions, bifunctional Ni- and Pt-based catalysts supported on Al₂O₃ and TiO₂ were evaluated under 30 bar hydrogen pressure at 250 °C. The inclusion of PVC, often regarded as a catalyst poison due to chlorine content, was examined at 1 wt% and 5 wt% to assess catalyst tolerance to it and resulted performance. Reaction rates and product selectivity were analyzed using gas chromatography. Results show that Ni/TiO₂ outperformed other catalysts, maintaining high activity and achieving up to 38.4% selectivity toward the C8–C16 SAF range with 5 wt% PVC, likely due to the strong chlorine affinity of the TiO₂ support that mitigates catalyst deactivation and enhances acidity. In contrast, Al₂O₃-supported catalysts experienced rate decline, likely due to active-site poisoning by chlorine. The work demonstrates the feasibility of using mixed plastic feedstocks with PVC for SAF production, offering a dual solution to waste management and sustainable fuel synthesis.

Research Sponsor

Dr. Linxiao Chen

First Reader

Dr. Bi-min Zhang Newby

Second Reader

Dr. Roya Gitiafroz

Honors Faculty Advisor

Dr. Bi-min Zhang Newby

Proprietary and/or Confidential Information

No

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